A recent study shines a spotlight on the development of covalent organic frameworks (COFs), particularly imine-linked varieties. Known for their tunable structure and remarkable stability, imine-linked COFs are set to revolutionize industries ranging from gas capture to advanced electronics. By focusing on the design and synthesis of these materials, the research offers valuable insights into the topology and creation of COF powders and thin films, promising to unlock new frontiers in technology and sustainability.